Projects

Concerted Proton Electron Transfer in Inorganic Synthesis and Catalyss; Towards Methane Valorisation

The CEPTr research program aims to isolate rare late transition element (TM) complexes with terminal oxo (O2-) ligands, using the combined electron and proton transfer as the lynchpin for their successful synthesis. Crucial to this endeavor is a new family of ligand scaffolds called f-CArAC (fused – Cyclic Aryl Amino Carbenes) which are able to support afore-mentioned complexes in both low and high oxidation states and with low coordination numbers.

Low Valent Bismuth Complexes for Small Molecule Activation

Low valent bismuth complexes have gathered much attention especially since their high-lying, partially occupied p-orbitals have the right symmetry, energy and occupancy to promote bond activation events in small molecules. In this respect, they mimic the d-orbitals of transition metal (TM) complexes that have historically dominated catalysis but are often toxic and/or rare and expensive. Furthermore, the rich redox chemistry of bismuth as well as the availability of both one and two reversible electron processes means that facile redox cycling, crucial to catalysis, is achievable.